title: Distribution and sources of polycyclic aromatic hydrocarbons (PAHs) in street dust from the Tokyo Metropolitan area.
abstract: Molecular distributions of polycyclic aromatic hydrocarbons (PAHs) in street dust samples collected from the Tokyo Metropolitan area were determined by capillary gas chromatography following HPLC fractionation. Three- to six-ring PAHs and sulfur-heterocyclics were detected. PAHs in the dusts were dominated by three and four unsubstituted ring systems with significant amounts of their alkyl homologues. PAHs were widely distributed in the streets, with concentrations (sigma COMB) of a few microgram/g dust. Automobile exhaust, asphalt, gasoline fuel, diesel fuel, tyre particles, automobile crankcase oils, and atmospheric fallout were also analysed. The PAH profile, especially the relative abundance of alkyl-PAHs and sulfur-containing heterocyclics, indicated that PAHs in the street dusts from roads carrying heavy traffic are mainly derived from automobile exhausts; dusts from residential areas have a more significant contribution from atmospheric fallout.
authors.affiliation: Department of Environmental Science and Conservation, Faculty of Agriculture, Tokyo University of Agriculture and Technology, Japan.
authors.forename: H
authors.initials: H
authors.lastname: Takada
authors.forename: T
authors.initials: T
authors.lastname: Onda
authors.forename: M
authors.initials: M
authors.lastname: Harada
authors.forename: N
authors.initials: N
authors.lastname: Ogura
mesh_terms: D002851:Chromatography, High Pressure Liquid / Q000379:methods; D004391:Dust / Q000032:analysis*; D004785:Environmental Pollutants / Q000032:analysis*; D006798:Housing; D006801:Humans; D011083:Polycyclic Compounds / Q000032:analysis*; D014041:Tokyo; D014186:Transportation; D014504:Urban Health
chemical_list: D004391:Dust; D004785:Environmental Pollutants; D011083:Polycyclic Compounds