title: Neutrons confirmed in Nagasaki and at the Army Pulsed Radiation Facility: implications for Hiroshima.
abstract: Recent reports have clearly demonstrated that large discrepancies exist between neutron activation measured in Hiroshima and activation calculated using the current dosimetry system, DS86. The reports confirmed previous results for cobalt activation in Hiroshima that suggested problems, and this has spurred a joint U.S.-Japan effort to identify the source(s) of this discrepancy. Here, new results are presented that appear to eliminate both the measurements of neutron activation and the DS86 air-transport calculations as potential sources of the discrepancy in Hiroshima. Computer transport of DS86 fission neutrons through large distances of air was validated using concrete samples from Nagasaki and chloride detectors placed at selected distances from a bare uranium reactor. In both cases, accelerator mass spectrometry was used to measure thermal neutron activation via the reaction, 35Cl(n, gamma)36Cl (half-life, 301,000 years). Good agreement was observed between measurements of neutron activation and DS86 calculations for Nagasaki, as well as for the reactor experiment. Thus the large discrepancy observed in Hiroshima appears not to be due to uncertainties in air-transport calculations or in the activation measurements; rather, the discrepancy appears to be due to uncertainties associated with the Hiroshima bomb itself.
authors.affiliation: Lawrence Livermore National Laboratory, Livermore, California 94550.
authors.forename: T
authors.initials: T
authors.lastname: Straume
authors.forename: L J
authors.initials: LJ
authors.lastname: Harris
authors.forename: A A
authors.initials: AA
authors.lastname: Marchetti
authors.forename: S D
authors.initials: SD
authors.lastname: Egbert
mesh_terms: D002712:Chlorides / Q000032:analysis; D003252:Construction Materials / Q000032:analysis* / Q000528:radiation effects; D007564:Japan; D009501:Neutron Activation Analysis / Q000379:methods; D009502:Neutrons; D009688:Nuclear Reactors; D009689:Nuclear Warfare; D011847:Radioactive Fallout / Q000032:analysis*; D012542:Scattering, Radiation
chemical_list: D002712:Chlorides; D011847:Radioactive Fallout