title: Transform-limited, narrow-linewidth lasing action in organic semiconductor microcavities
abstract: Lasing action in organic vertical-cavity surface-emitting laser (OVCSEL) structures is demonstrated. Optically pumped OVCSELs with an active layer composed of a thin-film organic semiconductor tris-(8-hydroxyquinoline) aluminum (Alq3) doped with DCM laser dye produced very narrow linewidth (0.2 +/- 0.1 angstrom), high-power (3 watts) emission that could be varied in different devices from orange to red. The efficient energy transfer from Alq3 to DCM results in a threshold input energy of 300 microjoules per square centimeter. An operational lifetime >10(6) laser pulses was achieved for a device operated well above threshold in atmosphere. The linewidths above threshold are Fourier transform-limited and could potentially be narrowed further.
authors.affiliation: Center for Photonics and Optoelectronic Materials (POEM), Department of Electrical Engineering and the Princeton Materials Institute, Princeton University, Princeton, NJ 08544, USA.
authors.initials: V
authors.lastname: Bulovic
authors.initials: VG
authors.lastname: Kozlov
authors.initials: VB
authors.lastname: Khalfin
authors.initials: SR
authors.lastname: Forrest