title: Heterodyne-detected fifth-order nonresonant Raman scattering from room temperature CS2.
abstract: Actively phase-locked heterodyne-detected fifth-order nonresonant Raman scattering from room temperature CS2 has been measured. The experimental signals have similar magnitudes, shapes, and sign changes as calculated responses obtained via molecular dynamics simulations [S. Saito and I. Ohmine, Phys. Rev. Lett. 88, 207401 (2002)]. The measured signals contain sign changes that appear to be associated with the coupling of rotational motions both to each other and to translational motions.
authors: Department of Chemistry, University of California, Berkeley, California 94720, USA.
authors: Laura J
authors: LJ
authors: Kaufman
authors: Jiyoung
authors: J
authors: Heo
authors: Larry D
authors: LD
authors: Ziegler
authors: Graham R
authors: GR
authors: Fleming