Characterisation of the thermally stimulated conductivity and thermoluminescence of natural topaz.
Thermally stimulated conductivity (TSC) and thermoluminescence (TL) measurements were conducted to investigate the mechanisms of charge transfer and luminescence emission in natural samples of Brazilian topaz irradiated with beta particles from a 90Sr/90Y source or with a 1.75 MeV Van de Graaff electron beam. The luminescence and conductivity were simultaneously monitored during the heating of the samples, allowing direct comparison of the TL and TSC peaks. The results show that the three main TL peaks are accompanied by corresponding TSC peaks, usually shifted to higher temperatures. Comparison of the relative TL/TSC intensities of peaks 2 and 3 indicates that the process of thermal quenching of the luminescence is probably active, which is also supported by TL/TSC measurements at different heating rates. Results on the dose response of TL/TSC peaks also reveal an interesting feature: the TL intensity shows a monotonic increase with dose in the range of study (50 Gy-3 kGy) comprising a linear-supralinear-saturation characteristic, while the TSC peaks exhibit an increase from 50 Gy to 1 kGy, followed by a small decrease for doses greater than 1 kGy. This result is interpreted in terms of a model involving multiple traps and one recombination centre.
Yukihara
E G
EG
Instituto de Física, Universidade de São Paulo, SP, Brazil. yukihara@thor.phy.okstate.edu
McKeever
S W S
SW
Okuno
E
E
Yoshimura
E M
EM
D000538:Aluminum Silicates / Q000737:chemistry / Q000528:radiation effects*; D001610:Beta Particles; D003460:Crystallization; D008163:Luminescent Measurements; D011854:Radiochemistry; D013814:Thermal Conductivity; D013819:Thermoluminescent Dosimetry / Q000379:methods* / Q000706:statistics & numerical data
D000538:Aluminum Silicates