Controlling the angular momentum composition of a Rydberg electron wave packet.
Sequences of phase-locked laser pulses have been employed to control the orbital angular momentum character of an electron wave packet, which is initially created from a superposition of s and d Rydberg series. By an intelligent choice of phase, which depends on the excitation energy and the quantum defects, we are able to selectively pump down either all or a fraction of one or other angular momentum component, and by employing multichannel quantum-defect theory we are able to analyze the quantum-state distribution in detail.
Verlet
J R R
JR
Department of Chemistry, King's College London, Strand, London WC2R 2LS, United Kingdom.
Stavros
V G
VG
Minns
R S
RS
Fielding
H H
HH