Theory of time-resolved photoelectron imaging: nonperturbative calculation for an internally converting polyatomic molecule.
We present the first calculation of time-resolved photoelectron angular distributions for a polyatomic system. Our method takes rotations into exact account, treats the laser field nonperturbatively, and computes the electronic dynamics from first principles. Our results point to the information content of time-resolved photoelectron imaging observables and illustrate the role played by the field intensity.
Suzuki
Yoshi-Ichi
Y
Steacie Institute for Molecular Science, National Research Council of Canada, Ottawa, Ontario, Canada K1A OR6.
Stener
Mauro
M
Seideman
Tamar
T