Persistent organic pollutants in air and vegetation from the Canadian Rocky Mountains.
The exchange of chlorinated organic pollutants between air and vegetation in cold, mountain environments was investigated through the extraction of coniferous vegetation and high-volume air samples collected from the Canadian Rocky Mountains during the summers of 1999 and 2000. Concentrations of several compounds in vegetation increased as temperatures decreased, whereas atmospheric concentrations were not related to temperature. Daily cycling of these compounds between air and vegetation as a result of diurnal temperature changes was not observed. Compared with concentrations in vegetation from the Canadian Rocky Mountains, plant samples from the western valley in British Columbia (Canada) showed higher pollutant levels. Chemical partitioning between vegetation and air was not correlated with temperature, indicating that air contamination is governed by long-range transport and not by local revolatilization events. Based on these observations, we show that both deposition at higher altitudes and long-range atmospheric transport influence chemical accumulation in vegetation from the Canadian Rocky Mountains.
Davidson
Deborah A
DA
Program for Chemical and Environmental Toxicology, Department of Biology, University of Ottawa, P.O. Box 450, Station A, Ottawa, Ontario KIN 6N5, Canada. deborah_anne_davidson@hc-sc.gc.ca
Wilkinson
Andrew C
AC
Kimpe
Lynda E
LE
Blais
Jules M
JM
D000393:Air Pollutants / Q000032:analysis*; D000416:Alberta; D001274:Atmospheric Pressure; D001955:British Columbia; D005591:Chemical Fractionation; D005843:Geography; D007306:Insecticides / Q000032:analysis*; D010944:Plants / Q000737:chemistry*; D011078:Polychlorinated Biphenyls / Q000032:analysis*; D013696:Temperature
D000393:Air Pollutants; D007306:Insecticides; D011078:Polychlorinated Biphenyls