Absolute ionization rates of multielectron transition metal atoms in strong infrared laser fields.
We report on nonresonant strong field ionization of the multielectron transition metal atoms V, Nb, Ta, Ni, and Pd. Operating in the adiabatic regime (lambda = 1.5 microm), we quantitatively determined both (i) the first charge state saturation intensities and (ii) the absolute ionization rates for intensities ranging from threshold up to 3 x 10(14) W/cm2. We observed a dramatic suppression of ionization relative to single active electron approximation expectations. We suggest that this derives from dynamic polarization or screening effects within the multielectron atom, stressing a need for many-body theories of strong field ionization.
Smits
Marc
M
Department of Physics and Astronomy, Vrije Universiteit Amsterdam, Netherlands.
de Lange
C A
CA
Stolow
Albert
A
Rayner
D M
DM