Incoherent subharmonic light scattering in isotropic media.
Incoherent subharmonic light scattering in isotropic media is a new kind of nonlinear light scattering, which involves single input photon and multiple output photons of equal frequency. We investigate theoretically the dependence of the subharmonic scattering intensity on the hyperpolarizability of molecules and the incident intensity using nonlinear optics theory similar to that used for Hyper-Rayleigh scattering and degenerate optical parametric oscillators. It is derived that the subharmonic scattering intensities grow exponentially or superexponentially with the hyperpolarizability of molecules and the incident intensity.
Feng
D H
DH
Laboratory for High Intensity Optics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, PR China. dhfeng@siom.ac.cn
Xu
Z Z
ZZ
Feng
X L
XL
Jia
T Q
TQ
Li
X X
XX
Liu
J S
JS
D008027:Light; D046911:Macromolecular Substances; D008956:Models, Chemical; D015233:Models, Statistical; D055095:Optics and Photonics; D017785:Photons; D012542:Scattering, Radiation; D013053:Spectrophotometry / Q000379:methods*
D046911:Macromolecular Substances