Mapping rotational coherences onto time-resolved photoelectron imaging observables.
We explore the information content of time-resolved photoelectron imaging, a potentially powerful pump-probe technique whose popularity has been rapidly growing in recent years. To that end, we identify a mapping of the alignment properties of time-evolving wave packets onto the moments of the photoelectron images and investigate its origin and consequences theoretically and numerically.
Suzuki
Yoshi-Ichi
Y
Chemical Dynamics Laboratory, RIKEN, Wako, Saitama 351-0198, Japan.
Seideman
Tamar
T