Franck-Condon blockade and giant Fano factors in transport through single molecules.
We show that Franck-Condon physics leads to a significant current suppression at low bias voltages (termed Franck-Condon blockade) in transport through single molecules with strong coupling between electronic and vibrational degrees of freedom. Transport in this regime is characterized by remarkably large Fano factors (10(2)-10(3) for realistic parameters), which arise due to avalanchelike transport of electrons. Avalanches occur in a self-similar manner over a wide range of time scales, leading to power-law dependences of the current noise on frequency and vibrational relaxation rate.
Koch
Jens
J
Institut für Theoretische Physik, Freie Universität Berlin, Arnimallee 14, 14195 Berlin, Germany.
von Oppen
Felix
F