title: Laser-induced incandescence study on the metal aerosol particles as the effect of the surrounding gas medium.
abstract: The fundamental heat transfer phenomena caused by the 1064 nm pulsed laser irradiations on the molybdenum aerosol particles were investigated by monitoring the time evolutions of the incandescence spectra using an ICCD detector with a multichannel spectrograph. The particle temperatures were evaluated from the incandescence spectra with the Planck function, and the cooling processes of the laser-heated particles were investigated. By measuring the decrease in the laser-heated particle temperatures with different surrounding media, the roles of the heat transfer processes such as vaporization, thermal radiation, and heat conduction to the surrounding media were discussed. The influences of the vaporization processes on the total heat transfer phenomena were investigated by monitoring the emissions of the constituent molybdenum atoms in the laser-induced incandescence spectra of the aerosol particles and also by investigating the relationships between the intensity of the incandescence and the fluence of the 1064 nm pulsed laser. The calculations using the theory of heat conduction suggested that the diameters of the particles produced by the photolysis of Mo(CO)6 depended on the nature of the surrounding gases.
authors.affiliation: Department of Chemistry, Nagaoka University of Technology, Nagaoka, Niigata 940-2188, Japan. murakami@chem.nagaokaut.ac.jp
authors.forename: Yoshinori
authors.initials: Y
authors.lastname: Murakami
authors.forename: Tsuyoshi
authors.initials: T
authors.lastname: Sugatani
authors.forename: Yoshio
authors.initials: Y
authors.lastname: Nosaka