title: The distribution and transport of Sellafield derived 137 Cs and 241 Am to western Irish Sea sediments.
abstract: Sellafield derived (137)Cs and (241)Am were analysed in surficial sediments at 23 sites in the western Irish Sea. Concentrations varied between 3-175 Bq (137)Cs/kg and 1-147 Bq (241)Am/kg. There are two distinct basins in the western Irish Sea separated by an area of restricted depth and this bathymetry is reflected in the radionuclide concentrations. Highest concentrations were found in the northerly samples and substantially lower concentrations further south. This pattern of distribution can be explained by the predominantly northerly residual flow and the existence of seasonal stratification in this area of weak tides. (137)Cs/(241)Am ratios were also highest in the northern basin, and it is suggested that this is caused by differences in the mechanisms of transport of the two elements. The direct physical migration of contaminated particles from the eastern Irish Sea is the dominant transport mechanism in the north of the study area, whereas transport in the dissolved phase is most important to the southern region. Concentrations of both elements were best correlated with the percentage <15 microm particulate fraction suggesting that particles within this range are most important for direct transport and scavenging from the soluble phase.
authors.affiliation: Department of Agriculture and Environmental Science, The Queens University of Belfast, Newforge Lane, Belfast BT9 5PX, Northern Ireland. mark.charlesworth@doeni.gov.uk
authors.forename: M E
authors.initials: ME
authors.lastname: Charlesworth
authors.forename: M
authors.initials: M
authors.lastname: Service
authors.forename: C E
authors.initials: CE
authors.lastname: Gibson
mesh_terms: D000576:Americium / Q000032:analysis*; D002588:Cesium Radioisotopes / Q000032:analysis*; D019015:Geologic Sediments / Q000032:analysis*; D009792:Oceans and Seas; D010316:Particle Size; D014872:Water Movements; D014875:Water Pollutants, Radioactive / Q000032:analysis*
chemical_list: D002588:Cesium Radioisotopes; D014875:Water Pollutants, Radioactive; D000576:Americium