Orientational kinetics of dipolar particles in a Maxwell fluid matrix: inertialess limit for the rotary microrheology.
We study magnetic response of an assembly of ferroparticles suspended in a viscoelastic matrix which is modeled by a Maxwell fluid with a unique stress relaxation time. The problem refers to the magnetic microrheology approach where deformational properties of a complex fluid are tested with the aid of embedded nanoparticle probes set to motion by an external ac magnetic field. A possibility is considered to simplify the description of the orientational kinetics of the system at the expense of neglecting inertia effects in particle rotary motion. It is shown that in this aspect a Maxwell matrix differs essentially from the Newtonian one. In the latter the inertialess approximation for the particles of the approximately 10nm size is valid practically unboundedly. For a viscoelastic matrix the inertialess approximation means an important restriction on the value of the stress relaxation time. Assuming weak nonequilibrium, the magneto-orientational relaxation times are found and low-frequency magnetic spectra of a viscoelastic suspension are determined in the presence of a constant (magnetizing) field.
Institute of Continuous Media Mechanics, Ural Branch of RAS, 614013, Perm, Russia. raikher@icmm.ru
Yu L
YL
Raikher
V V
VV
Rusakov