Predicting the long-time dynamic heterogeneity in a supercooled liquid on the basis of short-time heterogeneities.
We report that the local Debye-Waller factor in a simulated 2D glass-forming mixture exhibits significant spatial heterogeneities and that these short-time fluctuations provide an excellent predictor of the spatial distribution of the long-time dynamic propensities. In contrast, the potential energy per particle of the inherent structure does not correlate well with the spatially distributed dynamics.
Widmer-Cooper
Asaph
A
School of Chemistry, University of Sydney, Sydney, New South Wales 2006, Australia.
Harrowell
Peter
P