title: Size matters more than chemistry for cloud-nucleating ability of aerosol particles.
abstract: Size-resolved cloud condensation nuclei (CCN) spectra measured for various aerosol types at a non-urban site in Germany showed that CCN concentrations are mainly determined by the aerosol number size distribution. Distinct variations of CCN activation with particle chemical composition were observed but played a secondary role. When the temporal variation of chemical effects on CCN activation is neglected, variation in the size distribution alone explains 84 to 96% of the variation in CCN concentrations. Understanding that particles' ability to act as CCN is largely controlled by aerosol size rather than composition greatly facilitates the treatment of aerosol effects on cloud physics in regional and global models.
authors.affiliation: Department of Biogeochemistry, Max Planck Institute for Chemistry, Mainz 55128, Germany.
authors.forename: U
authors.initials: U
authors.lastname: Dusek
authors.forename: G P
authors.initials: GP
authors.lastname: Frank
authors.forename: L
authors.initials: L
authors.lastname: Hildebrandt
authors.forename: J
authors.initials: J
authors.lastname: Curtius
authors.forename: J
authors.initials: J
authors.lastname: Schneider
authors.forename: S
authors.initials: S
authors.lastname: Walter
authors.forename: D
authors.initials: D
authors.lastname: Chand
authors.forename: F
authors.initials: F
authors.lastname: Drewnick
authors.forename: S
authors.initials: S
authors.lastname: Hings
authors.forename: D
authors.initials: D
authors.lastname: Jung
authors.forename: S
authors.initials: S
authors.lastname: Borrmann
authors.forename: M O
authors.initials: MO
authors.lastname: Andreae