Magnetic properties of spin-orbital polarons in lightly doped cobaltates.
We present a numerical treatment of a spin-orbital-polaron model for NaxCoO2 at small hole concentration (0.7 < x 1). We demonstrate how the polarons account for the peculiar magnetic properties of this layered compound: They explain the large susceptibility; their internal degrees of freedom lead both to a negative Curie-Weiss temperature and yet to a ferromagnetic intralayer interaction, thereby resolving a puzzling contradiction between these observations. We make specific predictions on the momentum and energy location of excitations resulting from the internal degrees of freedom of the polaron, and discuss their impact on spin-wave damping.
Daghofer
M
M
Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, D-70569 Stuttgart, Germany.
Horsch
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Khaliullin
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