title: Effect of solids concentration distribution on the flue gas desulfurization process.
abstract: A dry flue gas desulfurization (FGD) process at 600-800 degrees C was studied in a pilot-scale circulating fluidized bed (CFB) experimental facility. Various fresh sorbent distribution types and internal structures were modeled numerically to investigate their effect on the gas-solid flow and sulfate reaction characteristics. Experimental results show that, after the fresh sorbent supply was stopped, the desulfurization efficiency declined rapidly even though the sorbent recirculation was maintained. Therefore, the fresh sorbent is the main contributor to the desulfurization process and the primary effect of the recirculated sorbent was to evenly distribute the fresh sorbent and to prolong the sorbent particle residence time. The numerical results demonstrate thatthe desulfurization efficiency varied greatly for the various fresh sorbent bottom injection methods. The desulfurization efficiency of the bottom-even injection method was 1.5 times that of the bottom two-sided injection method. Internal structures effectively improved the fresh sorbent solids concentration distribution and the desulfurization efficiency. Optimized internal structures increased the desulfurization efficiency of the bottom two-sided injection method by 46%, so that it was very close to that of the bottom-even injection method with only a 4.6% difference.
authors.affiliation: Key Laboratory for Thermal Science and Power Engineering of the Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, China.
authors.forename: Jie
authors.initials: J
authors.lastname: Zhang
authors.forename: Changfu
authors.initials: C
authors.lastname: You
authors.forename: Haiying
authors.initials: H
authors.lastname: Qi
authors.forename: Changhe
authors.initials: C
authors.lastname: Chen
authors.forename: Xuchang
authors.initials: X
authors.lastname: Xu
mesh_terms: D000327:Adsorption; D000393:Air Pollutants / Q000032:analysis / Q000737:chemistry; D017610:Calcium Compounds / Q000737:chemistry*; D002244:Carbon / Q000737:chemistry*; D003031:Coal; D060729:Coal Ash; D005740:Gases / Q000032:analysis / Q000737:chemistry; D017745:Incineration / Q000295:instrumentation / Q000379:methods*; D008855:Microscopy, Electron, Scanning; D008962:Models, Theoretical; D010087:Oxides / Q000737:chemistry*; D010316:Particle Size; D052638:Particulate Matter / Q000737:chemistry*; D013458:Sulfur Dioxide / Q000032:analysis / Q000737:chemistry*; D014867:Water / Q000737:chemistry*
chemical_list: D000393:Air Pollutants; D017610:Calcium Compounds; D003031:Coal; D060729:Coal Ash; D005740:Gases; D010087:Oxides; D052638:Particulate Matter; D014867:Water; D013458:Sulfur Dioxide; D002244:Carbon; C016538:lime