title: Radioactivity levels in aerosol particles surrounding a large TENORM waste repository after application of preliminary restoration work.
abstract: In this paper, (238)U-series radionuclides have been analysed in particulate matter samples collected at a phosphogypsum stack system located near the city of Huelva (SW Spain) during the course of 1 year. The results have been compared to those collected at a reference (background) site located a few km away, in order to establish if the stack system provokes an increase in radionuclide exposure due to inhalation with particulate matter. The (222)Rn progeny, which is considered a very important contributor to the internal dose rate received by the population, was collected for 6 months. The results indicate that for several types of radionuclides there is a significant increase in the radioactivity adsorbed by the aerosol particles collected at phosphogypsum stacks. The isotope analysis indicates that this increment could be affected by the water vapour emissions from the factory, which contain high concentrations of these radionuclides. However, the majority of these radionuclides could not be detected at the background location. The corresponding dose increment estimated at the sampling point is, however, negligible. This fact is a consequence of the very small radionuclide concentration increment, together with relatively conservative nature of the occupational factor applied. Regarding the Rn progeny, no significant differences between either the collecting sites has been registered due to of the dominant wind regime at the sampling locations.
authors.affiliation: Dpto. de Física Aplicada, Campus de El Carmen, University of Huelva, 21071 Huelva, Spain.
authors.forename: E
authors.initials: E
authors.lastname: Borrego
authors.forename: J L
authors.initials: JL
authors.lastname: Mas
authors.forename: J E
authors.initials: JE
authors.lastname: Martín
authors.forename: J P
authors.initials: JP
authors.lastname: Bolívar
authors.forename: F
authors.initials: F
authors.lastname: Vaca
authors.forename: J L
authors.initials: JL
authors.lastname: Aguado
mesh_terms: D002133:Calcium Sulfate / Q000737:chemistry; D052638:Particulate Matter / Q000032:analysis*; D010758:Phosphorus / Q000737:chemistry; D011834:Radiation Monitoring / Q000379:methods*; D011868:Radioisotopes / Q000032:analysis*; D012037:Refuse Disposal / Q000592:standards*; D012621:Seasons; D013030:Spain
chemical_list: D052638:Particulate Matter; D011868:Radioisotopes; C077769:phosphogypsum; D010758:Phosphorus; D002133:Calcium Sulfate