title: Modeling of SO(2) scrubbing in spray towers.
abstract: The present article aims at developing simple realistic models in order to describe the gaseous removal process of SO(2) by absorption with and without chemical reaction in spray towers. Effects of droplet size, droplet velocity, superficial gas velocity, liquid flow rate and tower height on the performance of such a system are theoretically predicted. Model calculations bring out some very interesting facets of gas scrubbing as functions of droplet diameter and velocity. Four distinct regimes, viz. droplet lean, dense droplet, rigid droplet and droplet inertia controlling regimes, are found important in spray scrubbing process. Model calculation also elucidates the existence of rigid droplet (sphere) for a distinct droplet size at a specific droplet velocity. Theoretical considerations reveal that best performance can be achieved in the droplet inertia-controlling regime. Effect of turbulence on scrubbing is also considered for modeling. The model development and experimental data are limited to use of water-soluble alkaline scrubbing. However, the predicted values agree reasonably well with the available experimental data at lower gas and liquid flow rates for relatively smaller droplets. Models can also be applied to any gas-liquid spray absorption process subject to the assumptions and conditions necessary to describe the specific physico-chemical hydrodynamics of the system. However, incorporation of various droplet interactions can further refine the models for better prediction of removal efficiency.
authors.affiliation: Department of Chemical Engineering, Indian Institute of Technology, Kharagpur, India. amitava.bandy@gmail.com
authors.forename: Amitava
authors.initials: A
authors.lastname: Bandyopadhyay
authors.forename: Manindra N
authors.initials: MN
authors.lastname: Biswas
mesh_terms: D000042:Absorption; D000393:Air Pollutants / Q000737:chemistry*; D000397:Air Pollution / Q000517:prevention & control*; D008962:Models, Theoretical; D015203:Reproducibility of Results; D012972:Sodium Hydroxide / Q000737:chemistry; D013458:Sulfur Dioxide / Q000737:chemistry*; D014867:Water / Q000737:chemistry
chemical_list: D000393:Air Pollutants; D014867:Water; D013458:Sulfur Dioxide; D012972:Sodium Hydroxide