Charge ordering and coexistence of charge fluctuations in quasi-two-dimensional organic conductors theta-(BEDT-TTF)2X.
We present a scenario for the peculiar coexistence of charge fluctuations observed in quasi-2D 1/4-filled organic conductors theta-(BEDT-TTF)2X in the quantum critical regime where the charge ordering is suppressed down to zero temperature. The scenario is explored in the extended Hubbard model including electron-phonon couplings on an anisotropic triangular lattice. We find that the coexisting fluctuations emerge from two different instabilities, the "Wigner crystallization on a lattice" driven by the off-site Coulomb repulsion and the charge-density-wave formation due to the nesting of the Fermi surface, not from phase competition or real-space inhomogeneity. This mechanism explains the contrastive temperature dependence of two fluctuations in experiments.
Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan.
Masafumi
M
Udagawa
Yukitoshi
Y
Motome