title: Sensitivities of ozone and fine particulate matter formation to emissions under the impact of potential future climate change.
abstract: Impact of climate change alone and in combination with currently planned emission control strategies are investigated to quantify effectiveness in decreasing regional ozone and PM2.5 over the continental U.S. using MM5, SMOKE, and CMAQ with DDM-3D. Sensitivities of ozone and PM2.5 formation to precursor emissions are found to change only slightly in response to climate change. In many cases, mass per ton sensitivities to NO(x) and SO2 controls are predicted to be greater in the future due to both the lower emissions as well as climate, suggesting that current control strategies based on reducing such emissions will continue to be effective in decreasing ground-level ozone and PM2.5 concentrations. SO2 emission controls are predicted to be most beneficial for decreasing summertime PM2.5 levels, whereas controls of NO(x) emissions are effective in winter. Spatial distributions of sensitivities are also found to be only slightly affected assuming no changes in land-use. Contributions of biogenic VOC emissions to PM2.5 formation are simulated to be more important in the future because of higher temperatures, higher biogenic emissions, and lower anthropogenic NO(x) and SO2 emissions.
authors.affiliation: School of Civil and Environmental Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332, USA.
authors.forename: Kuo-Jen
authors.initials: KJ
authors.lastname: Liao
authors.forename: Efthimios
authors.initials: E
authors.lastname: Tagaris
authors.forename: Kasemsan
authors.initials: K
authors.lastname: Manomaiphiboon
authors.forename: Sergey L
authors.initials: SL
authors.lastname: Napelenok
authors.forename: Jung-Hun
authors.initials: JH
authors.lastname: Woo
authors.forename: Shan
authors.initials: S
authors.lastname: He
authors.forename: Praveen
authors.initials: P
authors.lastname: Amar
authors.forename: Armistead G
authors.initials: AG
authors.lastname: Russell
mesh_terms: D002980:Climate; D010126:Ozone / Q000737:chemistry*; D010316:Particle Size
chemical_list: D010126:Ozone