title: Problems found using a radon stripping algorithm for retrospective assessment of air filter samples.
abstract: An evaluation of a large number of air sample filters was undertaken using a commercial alpha and beta spectroscopy system employing a passive implanted planar silicon (PIPS) detector. Samples were only measured after air flow through the filters had ceased. Use of a commercial radon stripping algorithm was implemented to discriminate anthropogenic alpha activity on the filters from the radon progeny. When uncontaminated air filters were evaluated, the results showed that there was a time-dependent bias in both average estimates and measurement dispersion of anthropogenic activity estimates with the relative bias being small compared to the dispersion, indicating that the system would not give false positive indications for an appropriately set decision level. By also measuring environmental air sample filters simultaneously with electroplated alpha sources, use of the radon stripping algorithm demonstrated a number of substantial unexpected deviations from calibrated values indicating that the system would give false negative indications. Use of the current algorithm is, therefore, not recommended for general assay applications. Use of the PIPS detector should only be utilized for gross counting without appropriate modifications to the curve-fitting algorithm. As a screening method, the radon stripping algorithm might be expected to see elevated alpha activities from pure Pu on air sample filters (not due to radon progeny) around the 200 disintegrations per minute level.
authors.affiliation: National Security Technologies, LLC, P.O. Box 98521, MS RSL-47, Las Vegas, NV 89193, USA. hayesrb@nv.doe.gov
authors.forename: Robert B
authors.initials: RB
authors.lastname: Hayes
mesh_terms: D000396:Air Pollutants, Radioactive / Q000032:analysis*; D000465:Algorithms; D005374:Filtration / Q000379:methods; D011834:Radiation Monitoring / Q000295:instrumentation / Q000379:methods*; D011886:Radon / Q000032:analysis*; D012984:Software
chemical_list: D000396:Air Pollutants, Radioactive; D011886:Radon