Collective oscillations in the classical nonlinear response of a chaotic system.
We establish a general semiquantitative phase-space picture of the classical nonlinear response in a strongly chaotic system. As opposed to the case of stable dynamics, the response functions decay exponentially at long times. Damped oscillations in response functions are attributed to collective resonances which do not correspond to any periodic classical motions. We calculate analytically the second-order response in a simple chaotic system and demonstrate the relevance of the concept for the interpretation of spectroscopic data.
Malinin
Sergey V
SV
Department of Chemistry, Wayne State University, 5101 Cass Avenue, Detroit, Michigan 48202, USA.
Chernyak
Vladimir Y
VY