title: Interannual variations in PM2.5 due to wildfires in the Western United States.
abstract: In this study we have evaluated the role of wildfires on concentrations of fine particle (d < 2.5 microm) organic carbon (OC) and particulate mass (PM2.5) in the Western United States for the period 1988-2004. To do this, we examined the relationship between mean summer PM2.5 and OC concentrations at 39 IMPROVE sites with a database of fires developed from federal fire reports. The gridded database of area burned was used to generate a database of biomass fuel burned using ecosystem-specific fuel loads. The OC, PM2.5, and fire data were evaluated for five regions: Northern Rocky Mountains (Region 1), Central Rocky Mountains (Region 2), Southwest (Region 3), California (Region 4), and Pacific Northwest (Region 5). In Regions 1, 2, and 5, we found good correlations of seasonal mean PM2.5 concentrations among the sites within each region. This indicates that a common influence was important in determining the PM concentration at all sites across each region. In Regions 1 and 2, we found a significant correlation between PM2.5 and both the area burned and biomassfuel burned in each region. This relationship is statistically significant using either the area burned or fuel burned, but the correlations are stronger using the biomass fuel burned. In all five regions we found a statistically significant relationship between biomass burned and organic carbon. Using these relationships, we can estimate the amount of PM2.5 due to fires in each region during summer. For the Regions 1 through 5, the average summer-long enhancement of PM2.5 due to fires is 1.84, 1.09, 0.61, 0.81, and 1.21 microg/m3, respectively, and approximately twice these values during large fire years.
authors.affiliation: University of Washington, Bothell, 18115 Campus Way NE, Bothell, Washington 98011, USA. djaffe@u.washington.edu
authors.forename: Dan
authors.initials: D
authors.lastname: Jaffe
authors.forename: William
authors.initials: W
authors.lastname: Hafner
authors.forename: Duli
authors.initials: D
authors.lastname: Chand
authors.forename: Anthony
authors.initials: A
authors.lastname: Westerling
authors.forename: Dominick
authors.initials: D
authors.lastname: Spracklen
mesh_terms: D000393:Air Pollutants / Q000032:analysis*; D002244:Carbon / Q000032:analysis; D004784:Environmental Monitoring; D005390:Fires; D010126:Ozone / Q000032:analysis; D010316:Particle Size; D052638:Particulate Matter / Q000032:analysis*; D012621:Seasons; D014481:United States
chemical_list: D000393:Air Pollutants; D052638:Particulate Matter; D010126:Ozone; D002244:Carbon