Control of four-level quantum coherence via discrete spectral shaping of an optical frequency comb.
We present experiments demonstrating high-resolution and wide-bandwidth coherent control of a four-level atomic system in a diamond configuration. A femtosecond frequency comb is used to excite a specific pair of two-photon transitions in cold 87Rb. The optical-phase-sensitive response of the closed-loop diamond system is studied by controlling the phase of the comb modes with a pulse shaper. Finally, the pulse shape is optimized resulting in a 256% increase in the two-photon transition rate by forcing constructive interference between the mode pairs detuned from an intermediate resonance.
Stowe
Matthew C
MC
JILA, National Institute of Standards and Technology and University of Colorado and Department of Physics, University of Colorado, Boulder, Colorado 80309-0440, USA.
Pe'er
Avi
A
Ye
Jun
J