title: Modification of the ultrasound induced activity by the presence of an electrode in a sonoreactor working at two low frequencies (20 and 40 kHz). Part I: Active zone visualization by laser tomography.
abstract: Sonoelectrochemical experiments differ from sonochemical ones by the introduction of electrodes in the sonicated reaction vessel. The aim of the study is to characterize the changes of the ultrasonic activity induced by the presence of an electrode located in front of the transducer. The scope of our investigations concerns two low frequencies vibration modes: 20 and 40 kHz. For this purpose, two laser visualization techniques have been used. The first part of the study, described in the present paper (part I), deals with the laser tomography technique which provides an accurate picture of the reactor actives zones, related to numerous cavitation events. For each frequency, two parameters were studied: the electrical power supplied to the transducer and the electrode transducer distance. At both frequencies, without electrode, we can observe distinct zones corresponding to cavitation production and stationary waves establishment. When increasing the input power, bubble clouds tend to form a unique cloud near the transducer. In presence of the electrode, bubble cavitation clouds are largely influenced by the obstacle. The second part of the paper (part II) will describe the Particle Image Velocimetry (P.I.V.) technique which allows to measure the velocity vector field in the fluid portion between the horn and the electrode.
authors.affiliation: Equipe SRS, Institut UTINAM/UMR 6213 CNRS Université de Franche-Comté, 30 avenue de l'Observatoire 25009 Besançon cedex, France.
authors.forename: A
authors.initials: A
authors.lastname: Mandroyan
authors.forename: R
authors.initials: R
authors.lastname: Viennet
authors.forename: Y
authors.initials: Y
authors.lastname: Bailly
authors.forename: M-L
authors.initials: ML
authors.lastname: Doche
authors.forename: J-Y
authors.initials: JY
authors.lastname: Hihn