title: Atmospheric dry deposition of polychlorinated dibenzo-p-dioxins and dibenzofurans in the vicinity of municipal solid waste incinerators.
abstract: This study focuses on the atmospheric dry deposition flux of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) in the vicinity of the two municipal solid waste incinerators (MSWIs) located in southern Taiwan. PCDD/Fs in ambient air were taken and analyzed for seventeen 2,3,7,8-substituted PCDD/Fs during November 2004 and July 2005. Results show that the mean concentrations of PCDD/Fs in the ambient air near MSWI-GS and MSWI-RW were 0.090 and 0.097pg I-TEQ/Nm(3), respectively. Dry deposition fluxes of total PCDD/Fs were 18.0 and 23.5pg I-TEQ/(m(2)d) in the ambient air near MSWI-GS and MSWI-RW, respectively, which were considerably higher than that measured in Guangzhou, China. Annual dry deposition fluxes of total PCDD/Fs in the ambient air near MSWI-GS and MSWI-RW were 189 and 217ng/(m(2)year), respectively, which were also much higher than dry deposition of total PCDD/Fs to the Atlantic Ocean. The results of the present study strongly suggest that exposure to PCDD/Fs in this area should be reduced. In addition, parametric sensitivity shows that dry deposition flux of PCDD/Fs is most sensitive to dry deposition velocity of the particle-phase, followed by air temperature and concentration of total suspended particulate but least sensitive to dry deposition velocity of the gas-phase.
authors.affiliation: Department of Environmental Engineering, National Cheng Kung University, Tainan 70101, Taiwan.
authors.forename: Yee-Lin
authors.initials: YL
authors.lastname: Wu
authors.forename: Long-Full
authors.initials: LF
authors.lastname: Lin
authors.forename: Lien-Te
authors.initials: LT
authors.lastname: Hsieh
authors.forename: Lin-Chi
authors.initials: LC
authors.lastname: Wang
authors.forename: Guo-Ping
authors.initials: GP
authors.lastname: Chang-Chien
mesh_terms: D000393:Air Pollutants / Q000032:analysis*; D001572:Benzofurans / Q000032:analysis*; D000072338:Dibenzofurans, Polychlorinated; D017745:Incineration; D000072317:Polychlorinated Dibenzodioxins / Q000031:analogs & derivatives* / Q000032:analysis; D011140:Polyurethanes / Q000032:analysis; D012037:Refuse Disposal; D012995:Solubility; D014887:Weather
chemical_list: D000393:Air Pollutants; D001572:Benzofurans; D000072338:Dibenzofurans, Polychlorinated; D000072317:Polychlorinated Dibenzodioxins; D011140:Polyurethanes