Nanosecond time-resolved investigations using the in situ of dynamic transmission electron microscope (DTEM).
Most biological processes, chemical reactions and materials dynamics occur at rates much faster than can be captured with standard video rate acquisition methods in transmission electron microscopes (TEM). Thus, there is a need to increase the temporal resolution in order to capture and understand salient features of these rapid materials processes. This paper details the development of a high-time resolution dynamic transmission electron microscope (DTEM) that captures dynamics in materials with nanosecond time resolution. The current DTEM performance, having a spatial resolution <10nm for single-shot imaging using 15ns electron pulses, will be discussed in the context of experimental investigations in solid state reactions of NiAl reactive multilayer films, the study of martensitic transformations in nanocrystalline Ti and the catalytic growth of Si nanowires. In addition, this paper will address the technical issues involved with high current, electron pulse operation and the near-term improvements to the electron optics, which will greatly improve the signal and spatial resolutions, and to the laser system, which will allow tailored specimen and photocathode drive conditions.
LaGrange
Thomas
T
Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, CA 94550, USA. lagrange@llnl.gov
Campbell
Geoffrey H
GH
Reed
B W
BW
Taheri
Mitra
M
Pesavento
J Bradley
JB
Kim
Judy S
JS
Browning
Nigel D
ND