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In the study of complex formation in aqueous solution by means of pH measurements, it is very useful to know the free ion concentrations in order to find each species composition and then calculate approximate values of their stability constants. From the pH determination alone, the unmeasured free ion concentrations can be calculated by a method in which a minimum number of integration and derivation steps are required. This process, called CILS, has been entirely computerized, and its conditions of application are illustrated with a simulated example.
Fournaise
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Laboratoire de Chimie de Coordination, Université de Reims Champagne-Ardenne, B.P. 347, 51062 Reims, France.
Petitfaux
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