Single-particle and collective mode couplings associated with 1- and 2-directional electronic ordering in metallic RTe3 (R=Ho,Dy,Tb).
The coupling of phonons with collective modes and single-particle gap excitations associated with one- (1d) and two-directional (2d) electronically driven charge-density wave (CDW) ordering in metallic RTe3 is investigated as a function of rare-earth ion chemical pressure (R=Tb,Dy,Ho) using femtosecond pump-probe spectroscopy. From the T dependence of the CDW gap DeltaCDW and the amplitude mode, we find that while the transition to a 1d-CDW ordered state at Tc1 initially proceeds in an exemplary mean-field-like fashion, below Tc1, DeltaCDW is depressed and departs from the mean-field behavior. The effect is apparently triggered by resonant mode mixing of the amplitude mode with a totally symmetric phonon at 1.75 THz. At low temperatures, when the state evolves into a 2d-CDW ordered state at Tc2 in the DyTe3 and HoTe3, additional much weaker mode mixing is evident but no soft mode is observed.
Yusupov
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Complex Matter Department, Jozef Stefan Institute, Jamova 39, 1000 Ljubljana, Slovenia. Roman.Yusupov@ijs.si
Mertelj
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Chu
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Fisher
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Mihailovic
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