Nuclear archeology in a bottle: evidence of pre-Trinity U.S. weapons activities from a waste burial site.
During World War II, the Hanford Site in Washington became the location for U.S. plutonium production. In 2004, a bottle containing a sample of plutonium was recovered from a Hanford waste trench. Here, state-of-the-art instrumental analyses, reactor model simulations, and investigative science techniques were used to provide insights as to the origin of this unknown sample, a process collectively termed as nuclear archeology. Isotopic age dating conducted on the sample in 2007 indicated the sample was separated from the spent fuel 61.6 +/- 4.5 years earlier. The isotope (22)Na, a detectable product of a secondary nuclear reaction, proved useful as a powerful tool for nuclear forensic analysis as (1) an easily detectable signifier of the presence of alpha emitting actinides, (2) an indicator of sample splitting, and (3) a measure of the time since sample splitting. Analytical results of minor actinide isotopes and reactor model simulations confirmed the material originated from the X-10 reactor in Oak Ridge, TN. Corroborated by historical documents, we concluded this sample was part of the first batch of Pu separated at T-Plant, Hanford, the world's first industrial-scale reprocessing facility, on December 9, 1944. This sample represents the oldest known collection of man-made (239)Pu in the world.
Schwantes
Jon M
JM
Pacific Northwest National Laboratory, P.O. Box 999, Richland, Washington 99352, USA. jon.schwantes@pnl.gov
Douglas
Matthew
M
Bonde
Steven E
SE
Briggs
James D
JD
Farmer
Orville T
OT
Greenwood
Lawrence R
LR
Lepel
Elwood A
EA
Orton
Christopher R
CR
Wacker
John F
JF
Luksic
Andrzej T
AT