title: Convergent radial tracing of viral and solute transport in gneiss saprolite.
abstract: Deeply weathered crystalline rock aquifer systems comprising unconsolidated saprolite and underlying fractured bedrock (saprock) underlie 40% of sub-Saharan Africa. The vulnerability of this aquifer system to contamination, particularly in rapidly urbanizing areas, remains poorly understood. In order to assess solute and viral transport in saprolite derived from Precambrian gneiss, forced-gradient tracer experiments using chloride and Escherichia coli phage PhiX174 were conducted in southeastern Uganda. The bacteriophage tracer was largely unrecovered; adsorption to the weathered crystalline rock matrix is inferred and enabled by the low pH (5.7) of site ground water and the bacteriophage's relatively high isoelectric point (pI = 6.6). Detection of the applied PhiX174 phage in the pumping well discharge at early times during the experiment traces showed, however, that average ground water flow velocities exceed that of the inert solute tracer, chloride. This latter finding is consistent with observations in other hydrogeological environments where statistically extreme sets of microscopic flow velocities are considered to transport low numbers of fecal pathogens and their proxies along a selected range of linked ground water pathways. Application of a radial advection-dispersion model with an exponentially decaying source term to the recovered chloride tracer estimates a dispersivity (alpha) of 0.8 +/- 0.1 m over a distance of 4.15 m. Specific yield (S(y)) is estimated to be 0.02 from volume balance calculations based on tracer experiments. As single-site observations, our estimates of saprolite S(y) and alpha are tentative but provide a starting point for assessing the vulnerability of saprolite aquifers in sub-Saharan Africa to contamination and estimating quantitatively the impact of climate and abstraction on ground water storage.
authors.affiliation: Department of Geography, University College London, Gower St., London WC1E 6BT, UK. r.taylor@geog.ucl.ac.uk
authors.forename: Richard
authors.initials: R
authors.lastname: Taylor
authors.forename: Callist
authors.initials: C
authors.lastname: Tindimugaya
authors.forename: John
authors.initials: J
authors.lastname: Barker
authors.forename: David
authors.initials: D
authors.lastname: Macdonald
authors.forename: Robinah
authors.initials: R
authors.lastname: Kulabako
mesh_terms: D017954:Africa South of the Sahara; D004784:Environmental Monitoring; D019015:Geologic Sediments; D014454:Uganda; D014872:Water Movements