Direct observation of a nuclear spin excitation in Ho2Ti2O7.
A single nondispersive excitation is observed by means of neutron backscattering, at E_{0}=26.3 microeV in the spin ice Ho2Ti2O7 but not in the isotopically enriched 162Dy2Ti2O7 analogue. The intensity of this excitation is rather small, less, similar0.2% of the elastic intensity. It is clearly observed below 80 K but resolution limited only below approximately 65 K. The application of a magnetic field up to micro_{0}H=4.5 T, at 1.6 K, has no measurable effect on the energy or intensity. This nuclear excitation is believed to perturb the electronic, Ising spin system resulting in the persistent spin dynamics observed in spin ice compounds.
Ehlers
G
G
Spallation Neutron Source, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831-6475, USA.
Mamontov
E
E
Zamponi
M
M
Kam
K C
KC
Gardner
J S
JS