Comparison study of supercontinuum generation by molecular alignment of N2 and O2.
We study the supercontinuum generation through femtosecond filamentation by using the quantum wake of the prealigned diatomic molecules of O(2) and N(2), where significant ultraviolet extension of the generated supercontinuum is attributed to the additional cross-focusing effect around parallel revival of molecular alignment and the consequent self-steepening as well as space-time focusing effect. Due to the discrepancy of the polarizabilities between O(2) and N(2) molecules, the spectral ultraviolet extension of the generated supercontinuum is more noticeable in molecular O(2) than that in N(2), and an extended supercontinuum spectrum from 370 to 900 nm is observed in O(2) of 2 atm. The detailed dependence of the generated supercontinuum on the pump intensity for molecular alignment and gas pressure of O(2) and N(2) molecules are performed.
Cai
Hua
H
State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai , China.
Wu
Jian
J
Peng
Yan
Y
Zeng
Heping
H