title: Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode.
abstract: Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented.
authors.forename: Wolfgang
authors.initials: W
authors.lastname: Wagner
authors.forename: Chunqiang
authors.initials: C
authors.lastname: Li
authors.forename: John
authors.initials: J
authors.lastname: Semmlow
authors.forename: Warren
authors.initials: W
authors.lastname: Warren