title: Spatial control of 3D energy transfer in supramolecular nanostructured host-guest architectures.
abstract: Systematic control of 3D energy transfer (ET) dynamics is achieved in supramolecular nanostructured host-guest systems using spacer-functionalized guest chromophores. Quantum chemistry-based Monte Carlo simulations reveal the strong impact of the spacer length on the ET dynamics, efficiency, and dimensionality. Remarkably high exciton diffusion lengths demonstrate that there is ample scope for optimizing oligomeric or polymeric optoelectronic devices.
authors: Lucas
authors: L
authors: Viani
authors: Lars Poulsen
authors: LP
authors: Tolbod
authors: Mikael
authors: M
authors: Jazdzyk
authors: Greta
authors: G
authors: Patrinoiu
authors: Fabrizio
authors: F
authors: Cordella
authors: Andrea
authors: A
authors: Mura
authors: Giovanni
authors: G
authors: Bongiovanni
authors: Chiara
authors: C
authors: Botta
authors: David
authors: D
authors: Beljonne
authors: Jérôme
authors: J
authors: Cornil
authors: Michael
authors: M
authors: Hanack
authors: Hans-Joachim
authors: HJ
authors: Egelhaaf
authors: Johannes
authors: J
authors: Gierschner
mesh_terms: D004735:Energy Transfer; D008958:Models, Molecular; D015394:Molecular Structure; D049329:Nanostructures / Q000737:chemistry*; D011789:Quantum Theory; D013343:Styrenes / Q000737:chemistry
chemical_list: D013343:Styrenes; C507243:distyrylbenzene