title: Proposed triaxial atomic force microscope contact-free tweezers for nanoassembly.
abstract: We propose a triaxial atomic force microscope contact-free tweezer (TACT) for the controlled assembly of nanoparticles suspended in a liquid. The TACT overcomes four major challenges faced in nanoassembly, as follows. (1) The TACT can hold and position a single nanoparticle with spatial accuracy smaller than the nanoparticle size (approximately 5 nm). (2) The nanoparticle is held away from the surface of the TACT by negative dielectrophoresis to prevent van der Waals forces from making it stick to the TACT. (3) The TACT holds nanoparticles in a trap that is size-matched to the particle and surrounded by a repulsive region so that it will only trap a single particle at a time. (4) The trap can hold a semiconductor nanoparticle in water with a trapping energy greater than the thermal energy. For example, a 5 nm radius silicon nanoparticle is held with 10 k(B)T at room temperature. We propose methods for using the TACT as a nanoscale pick-and-place tool to assemble semiconductor quantum dots, biological molecules, semiconductor nanowires, and carbon nanotubes.
authors.affiliation: School of Engineering and Applied Science, Harvard University, Cambridge, MA 02138, USA.
authors.forename: Keith A
authors.initials: KA
authors.lastname: Brown
authors.forename: Robert M
authors.initials: RM
authors.lastname: Westervelt
mesh_terms: D000465:Algorithms; D055590:Electromagnetic Phenomena; D004867:Equipment Design; D018625:Microscopy, Atomic Force / Q000295:instrumentation / Q000379:methods*; D053758:Nanoparticles / Q000737:chemistry*; D036103:Nanotechnology / Q000379:methods*; D045663:Quantum Dots