A hierarchical Fe/ZSM-5 zeolite with superior catalytic performance for benzene hydroxylation to phenol.
We report the one-step synthesis of a highly active hierarchical Fe/ZSM-5 zeolite catalyst with a strongly improved lifetime in the selective hydroxylation of benzene to phenol with nitrous oxide; compared to the best Fe/ZSM-5 catalyst, the turnover number after 24 h on stream is almost four times higher.
Xin
Hongchuan
H
State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian, China.
Koekkoek
Arjan
A
Yang
Qihua
Q
van Santen
Rutger
R
Li
Can
C
Hensen
Emiel J M
EJ