title: A hierarchical Fe/ZSM-5 zeolite with superior catalytic performance for benzene hydroxylation to phenol.
abstract: We report the one-step synthesis of a highly active hierarchical Fe/ZSM-5 zeolite catalyst with a strongly improved lifetime in the selective hydroxylation of benzene to phenol with nitrous oxide; compared to the best Fe/ZSM-5 catalyst, the turnover number after 24 h on stream is almost four times higher.
authors.affiliation: State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian, China.
authors.forename: Hongchuan
authors.initials: H
authors.lastname: Xin
authors.forename: Arjan
authors.initials: A
authors.lastname: Koekkoek
authors.forename: Qihua
authors.initials: Q
authors.lastname: Yang
authors.forename: Rutger
authors.initials: R
authors.lastname: van Santen
authors.forename: Can
authors.initials: C
authors.lastname: Li
authors.forename: Emiel J M
authors.initials: EJ
authors.lastname: Hensen