Observation of the dynamic Jahn-Teller effect in the excited states of nitrogen-vacancy centers in diamond.
The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Interexcited state population relaxation is shown to broaden the zero-phonon line and both the relaxation and linewidth are found to follow a T(5) dependence for T < 100 K. This dependence indicates that the dynamic Jahn-Teller effect is the dominant dephasing mechanism for the NV optical transitions at low temperatures.
Fu
Kai-Mei C
KM
Information and Quantum Systems Lab, Hewlett-Packard Laboratories, 1501 Page Mill Road, MS1123, Palo Alto, California 94304, USA. kai-mei.fu@hp.com
Santori
Charles
C
Barclay
Paul E
PE
Rogers
Lachlan J
LJ
Manson
Neil B
NB
Beausoleil
Raymond G
RG