Hybrid gap modes induced by fiber taper waveguides: application in spectroscopy of single solid-state emitters deposited on thin films.
We show, via simulations, that an optical fiber taper waveguide can be an efficient tool for photoluminescence and resonant, extinction spectroscopy of single emitters, such as molecules or colloidal quantum dots, deposited on the surface of a thin dielectric membrane. Placed over a high refractive index membrane, a tapered fiber waveguide induces the formation of hybrid mode waves, akin to dielectric slotted waveguide modes, that provide strong field confinement in the low index gap region. The availability of such gap-confined waves yields potentially high spontaneous emission enhancement factors (approximately 20), fluorescence collection efficiencies (approximately 23%), and transmission extinction (approximately 20%) levels. A factor of two improvement in fluorescence and extinction levels is predicted if the membrane is instead replaced with a suspended channel waveguide. Two configurations, for operation in the visible (approximately 600 nm) and near-infrared (approximately 1300 nm) spectral ranges are evaluated, presenting similar performances.
Davanço
Marcelo
M
1Center for Nanoscale Science and Technology, National Institute of Standards and Technology, Gaithersburg, MD, USA. mdavanco@nist.gov
Srinivasan
Kartik
K
D017076:Computer-Aided Design; D004735:Energy Transfer; D004867:Equipment Design; D019544:Equipment Failure Analysis; D005336:Fiber Optic Technology / Q000295:instrumentation*; D008029:Lighting / Q000295:instrumentation*; D015203:Reproducibility of Results; D012666:Semiconductors; D012680:Sensitivity and Specificity; D013057:Spectrum Analysis / Q000379:methods*