Field-induced control of universal fluorescence intermittency of a quantum dot light emitter.
With the nonstochastic quantum mechanical study of a quantum dot light emitter, we find that fluorescence intermittency statistics are universal and insensitive to the microscopic nature of the tunneling fluctuation between quantum dot and trapping state. We also investigate the power-law exponent theta and the crossover time tau(C) of the on-time (tau(on)) probability P(tau(on)) proportional to tau(on) (-theta) (for tau(on) less than or approximately equal tau(C)) and proportional to e(-Gamma)tau(on) ) (for tau(on) greater than or approximately equal tau(C)) under an optical field of given energy and strength. For easy off-resonance excitation, it is found in both numerical and analytic ways that tau(C) (-1) is proportional to the intensity of the optical field (i.e., the square of the field strength) independent of the internal parameters of a quantum dot. Furthermore, it is also found that theta=2 in the limit of vanishing field strength is the upper bound of the exponent and theta becomes less than 2 as the field strength increases.
Lee
J D
JD
School of Materials Science, Japan Advanced Institute of Science and Technology, Ishikawa 923-1292, Japan. jdlee@jaist.ac.jp
Maenosono
S
S