Optical properties of (SrMnO₃)n/(LaMnO₃)₂n superlattices: an insulator-to-metal transition observed in the absence of disorder.
We measure the optical conductivity, σ1(ω), of (SrMnO3)n/(LaMnO3)2n superlattices (SL) for n = 1, 3, 5, and 8 and 10 < T < 400 K. Data show a T-dependent insulator to metal transition (IMT) for n ≤ 3, driven by the softening of a polaronic mid-infrared band. At n = 5 that softening is incomplete, while at the largest-period n = 8 compound the MIR band is independent of T and the SL remains insulating. One can thus first observe the IMT in a Manganite system in the absence of the disorder due to chemical doping. Unsuccessful reconstruction of the SL optical properties from those of the original bulk materials suggests that (SrMnO3)n/(LaMnO3)2n heterostructures give rise to a novel electronic state.
Sincrotrone Trieste, Area Science Park, I-34012 Trieste, Italy.
Andrea
A
Perucchi
Leonetta
L
Baldassarre
Alessandro
A
Nucara
Paolo
P
Calvani
Carolina
C
Adamo
Darrell G
DG
Schlom
Pasquale
P
Orgiani
Luigi
L
Maritato
Stefano
S
Lupi