title: Temporal variation of oxygen isotope ratios (δ18O) in drinking water: implications for specifying location of origin with human scalp hair.
abstract: Previous work suggests that δ(18)O values of human hair can be used to constrain the region-of-origin of unknown individuals, but robust assessments of uncertainties in this method are lacking. Here we assess one source of uncertainty - temporal variation in the δ(18)O value of drinking water - using a monthly tap water survey of δ(18)O to develop geospatial models (i.e., maps) of the intra-annual variation (seasonality) in tap water δ(18)O for the contiguous USA. Temporal variation in tap water δ(18)O was correlated with water-supply type, and was related to geographic patterns of precipitation δ(18)O seasonality and water residence time. The maps were applied in a Bayesian framework to identify the geographic origin of an unidentified woman found in Utah, based on measured δ(18)O of scalp hair. The results are robust in specifying parts of the western USA as the most likely region-of-origin. Incorporation of tap water δ(18)O seasonality in the analysis reduces the precision of geographic assignments, but other sources of uncertainty (e.g., spatial interpolation uncertainty) have an equal or larger effect.
authors.affiliation: Purdue University, Department of Earth and Atmospheric Sciences, West Lafayette, IN 47907-2051, USA. cdkennedy@purdue.edu
authors.forename: Casey D
authors.initials: CD
authors.lastname: Kennedy
authors.forename: Gabriel J
authors.initials: GJ
authors.lastname: Bowen
authors.forename: James R
authors.initials: JR
authors.lastname: Ehleringer
mesh_terms: D000704:Analysis of Variance; D001499:Bayes Theorem; D005260:Female; D044707:Forensic Sciences; D005843:Geography; D006197:Hair / Q000737:chemistry*; D006801:Humans; D015233:Models, Statistical; D010103:Oxygen Isotopes / Q000032:analysis*; D011891:Rain; D012621:Seasons; D014481:United States; D014867:Water / Q000737:chemistry*; D014881:Water Supply
chemical_list: D010103:Oxygen Isotopes; D014867:Water