title: Reactor-based management of used nuclear fuel: assessment of major options.
abstract: This paper discusses the current status of the ongoing Advanced Fuel Cycle Initiative (AFCI) program in the U.S. Department of Energy that is investigating the potential for using the processing and recycling of used nuclear fuel to improve radioactive waste management, including used fuel. A key element of the strategies is to use nuclear reactors for further irradiation of recovered chemical elements to transmute certain long-lived highly-radioactive isotopes into less hazardous isotopes. Both thermal and fast neutron spectrum reactors are being studied as part of integrated nuclear energy systems where separations, transmutation, and disposal are considered. Radiotoxicity is being used as one of the metrics for estimating the hazard of used fuel and the processing of wastes resulting from separations and recycle-fuel fabrication. Decay heat from the used fuel and/or wastes destined for disposal is used as a metric for use of a geologic repository. Results to date indicate that the most promising options appear to be those using fast reactors in a repeated recycle mode to limit buildup of higher actinides, since the transuranic elements are a key contributor to the radiotoxicity and decay heat. Using such an approach, there could be much lower environmental impact from the high-level waste as compared to direct disposal of the used fuel, but there would likely be greater generation of low-level wastes that will also require disposal. An additional potential waste management benefit is having the ability to tailor waste forms and contents to one or more targeted disposal environments (i.e., to be able to put waste in environments best-suited for the waste contents and forms).
authors.affiliation: Idaho National Laboratory, P.O. Box 1625, Mail Stop 3860, Idaho Falls, ID 83415-3860, USA. phillip.finck@inl.gov
authors.forename: Phillip J
authors.initials: PJ
authors.lastname: Finck
authors.forename: Roald A
authors.initials: RA
authors.lastname: Wigeland
authors.forename: Robert N
authors.initials: RN
authors.lastname: Hill
mesh_terms: D006077:Government Agencies / Q000706:statistics & numerical data; D006358:Hot Temperature; D009688:Nuclear Reactors; D011850:Radioactive Waste; D011854:Radiochemistry; D011868:Radioisotopes / Q000737:chemistry / Q000633:toxicity; D014481:United States; D018505:Waste Management / Q000295:instrumentation* / Q000379:methods* / Q000706:statistics & numerical data
chemical_list: D011850:Radioactive Waste; D011868:Radioisotopes