title: Communication: Interfacial water structure revealed by ultrafast two-dimensional surface vibrational spectroscopy.
abstract: Knowledge of the interfacial water structure is essential for a basic understanding of the many environmental, technological, and biophysical systems in which aqueous interfaces appear. Using ultrafast two-dimensional surface-specific vibrational spectroscopy we show that the structure of heavy water at the water-air interface displays short-lived heterogeneity and is very different from that at the water-lipid interface.
authors.affiliation: FOM-Institute AMOLF, Science Park 104, 1098 XG Amsterdam, The Netherlands.
authors.forename: Zhen
authors.initials: Z
authors.lastname: Zhang
authors.forename: Lukasz
authors.initials: L
authors.lastname: Piatkowski
authors.forename: Huib J
authors.initials: HJ
authors.lastname: Bakker
authors.forename: Mischa
authors.initials: M
authors.lastname: Bonn