title: Probing the timescale of the exchange interaction in a ferromagnetic alloy.
abstract: The underlying physics of all ferromagnetic behavior is the cooperative interaction between individual atomic magnetic moments that results in a macroscopic magnetization. In this work, we use extreme ultraviolet pulses from high-harmonic generation as an element-specific probe of ultrafast, optically driven, demagnetization in a ferromagnetic Fe-Ni alloy (permalloy). We show that for times shorter than the characteristic timescale for exchange coupling, the magnetization of Fe quenches more strongly than that of Ni. Then as the Fe moments start to randomize, the strong ferromagnetic exchange interaction induces further demagnetization in Ni, with a characteristic delay determined by the strength of the exchange interaction. We can further enhance this delay by lowering the exchange energy by diluting the permalloy with Cu. This measurement probes how the fundamental quantum mechanical exchange coupling between Fe and Ni in magnetic materials influences magnetic switching dynamics in ferromagnetic materials relevant to next-generation data storage technologies.
authors.affiliation: Department of Physics and JILA, University of Colorado, Boulder, CO 80309-0440, USA. smathias@jila.colorado.edu
authors.forename: Stefan
authors.initials: S
authors.lastname: Mathias
authors.forename: Chan
authors.initials: C
authors.lastname: La-O-Vorakiat
authors.forename: Patrik
authors.initials: P
authors.lastname: Grychtol
authors.forename: Patrick
authors.initials: P
authors.lastname: Granitzka
authors.forename: Emrah
authors.initials: E
authors.lastname: Turgut
authors.forename: Justin M
authors.initials: JM
authors.lastname: Shaw
authors.forename: Roman
authors.initials: R
authors.lastname: Adam
authors.forename: Hans T
authors.initials: HT
authors.lastname: Nembach
authors.forename: Mark E
authors.initials: ME
authors.lastname: Siemens
authors.forename: Steffen
authors.initials: S
authors.lastname: Eich
authors.forename: Claus M
authors.initials: CM
authors.lastname: Schneider
authors.forename: Thomas J
authors.initials: TJ
authors.lastname: Silva
authors.forename: Martin
authors.initials: M
authors.lastname: Aeschlimann
authors.forename: Margaret M
authors.initials: MM
authors.lastname: Murnane
authors.forename: Henry C
authors.initials: HC
authors.lastname: Kapteyn