Nanowire heating by optical electromagnetic irradiation.
The dissipative absorption of electromagnetic energy by 1D nanoscale structures at optical frequencies is applicable to several important phenomena, including biomedical photothermal theranostics, nanoscale photovoltaic materials, atmospheric aerosols, and integrated photonic devices. Closed-form analytical calculations are presented for the temperature rise within infinite circular cylinders with nanometer-scale diameters (nanowires) that are irradiated at right angles by a continuous-wave laser source polarized along the nanowire's axis. Solutions for the heat source are compared to both numerical finite-difference time domain (FDTD) simulations and well-known Mie scattering cross sections for infinite cylinders. The analysis predicts that the maximum temperature increase is affected not only by the cylinder's composition and porosity but also by morphology-dependent resonances (MDRs) that lead to significant spikes in the local temperature at particular diameters. Furthermore, silicon nanowires with high thermal conductivities are observed to exhibit extremely uniform internal temperatures during electromagnetic heating to 1 part in 10(6), including cases where there are substantial fluctuations of the internal electric-field source term that generates the Joule heating. For a highly absorbing material such as carbon, much higher temperatures are predicted, the internal temperature distribution is nonuniform, and MDRs are not encountered.
Department of Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States.
Paden B
PB
Roder
Peter J
PJ
Pauzauskie
E James
EJ
Davis
D055590:Electromagnetic Phenomena; D006358:Hot Temperature; D007834:Lasers; D053770:Nanowires; D055095:Optics and Photonics; D012825:Silicon; D013696:Temperature
D012825:Silicon