title: Quantum stochastic dynamics in the presence of a time-periodic rapidly oscillating potential: nonadiabatic escape rate.
abstract: Escape from a metastable state in the presence of a high-frequency field (where the driving becomes nonadiabatic) underlies a broad range of phenomena of physics and chemistry, and thus its understanding is of paramount importance. We study the problem of intermediate-to-high-damping escape from a metastable state of a dissipative system driven by a rapidly oscillating field, one of the most important classes of nonequilibrium systems, in a broad range of field driving frequencies (ω) and amplitudes (a). We construct a Langevin equation using quantum gauge transformation in the light of Floquet theorem and exploiting a systematic perturbative expansion in powers of 1/ω using "Kapitza-Landau time window". The quantum dynamics in a high-frequency field are found to be described by an effective time-independent potential. The temperature dependence of escape rate and the change of its form with varying parameters of the field have been analyzed. It may decrease upon increasing the temperature which is contingent on the effects of intricate interplay between external modulation and dissipation. The crossover temperature between tunnelling and thermal hopping increases with an increase in external modulation so that quantum effects in the escape are relevant at higher temperatures. These observations are uncommon and counterintuitive and, therefore, of considerable interest. Our results might be valuable for the exploration of the dynamics of cold atoms in electromagnetic fields.
authors.affiliation: Department of Chemistry, Bengal Engineering and Science University , Shibpur, Howrah 711103, India.
authors.forename: Anindita
authors.initials: A
authors.lastname: Shit
authors.forename: Sudip
authors.initials: S
authors.lastname: Chattopadhyay
authors.forename: Jyotipratim Ray
authors.initials: JR
authors.lastname: Chaudhuri
mesh_terms: D009038:Motion; D011789:Quantum Theory; D013269:Stochastic Processes; D013696:Temperature; D013997:Time Factors