title: Use of a multichannel collimator for structural investigation of low-Z dense liquids in a diamond anvil cell: validation on fluid H2 up to 5 GPa.
abstract: We report the first application of a multichannel collimator (MCC) to perform quantitative structure factor measurements of dense low-Z fluids in a diamond anvil cell (DAC) using synchrotron x-ray diffraction. The MCC design, initially developed for the Paris-Edinburgh large volume press geometry, has been modified for use with diamond anvil cells. A good selectivity of the diffracted signal of the dense fluid sample is obtained due to a large rejection of the Compton diffusion from the diamond anvils. The signal to background ratio is significantly improved. We modify previously developed analytical techniques for quantitative measurement of the structure factor of fluids in DACs [J. H. Eggert, G. Weck, P. Loubeyre, and M. Mezouar, Phys. Rev. B 65, 174105 (2002)] to account for the contribution of the MCC. We present experimental results on liquids argon and hydrogen at 296 K to validate our method and test its limits, respectively.
authors.affiliation: CEA, DAM, DIF, 91297 Arpajon, France.
authors.forename: Gunnar
authors.initials: G
authors.lastname: Weck
authors.forename: Gaston
authors.initials: G
authors.lastname: Garbarino
authors.forename: Sandra
authors.initials: S
authors.lastname: Ninet
authors.forename: Dylan
authors.initials: D
authors.lastname: Spaulding
authors.forename: Frederic
authors.initials: F
authors.lastname: Datchi
authors.forename: Paul
authors.initials: P
authors.lastname: Loubeyre
authors.forename: Mohamed
authors.initials: M
authors.lastname: Mezouar