title: Neutron scattering and μSR investigations of the low temperature state of LuCuGaO₄.
abstract: LuCuGaO₄ has magnetic Cu(2+) and diamagnetic Ga(3+) ions distributed on a triangular bilayer and is suggested to undergo a spin glass transition at Tg ∼ 0.4 K. Using μSR (muon spin rotation) and neutron scattering measurements, we show that at low temperature the spins form a short range correlated state with spin fluctuations detectable over a wide range of timescales: at 0.05 K magnetic fluctuations can be detected in both the μSR time window and also extending beyond 7 meV in the inelastic neutron scattering response, indicating magnetic fluctuations spanning timescales between ∼10(-5) and ∼10(-10) s. The dynamical susceptibility scales according to the form χ″(ω)T(α), with α = 1, throughout the measured temperature range (0.05-50 K). These effects are associated with quantum fluctuations and some degree of structural disorder in ostensibly quite different materials, including certain heavy fermion alloys, kagome spin liquids, quantum spin glasses, and valence bond glasses. We therefore suggest that LuCuGaO₄ is an interesting model compound for the further examination of disorder and quantum magnetism.
authors.affiliation: Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA.
authors.forename: S
authors.initials: S
authors.lastname: Calder
authors.forename: S R
authors.initials: SR
authors.lastname: Giblin
authors.forename: D R
authors.initials: DR
authors.lastname: Parker
authors.forename: P P
authors.initials: PP
authors.lastname: Deen
authors.forename: C
authors.initials: C
authors.lastname: Ritter
authors.forename: J R
authors.initials: JR
authors.lastname: Stewart
authors.forename: S
authors.initials: S
authors.lastname: Rols
authors.forename: T
authors.initials: T
authors.lastname: Fennell
mesh_terms: D008187:Lutetium / Q000737:chemistry*; D008422:Materials Testing; D053758:Nanoparticles / Q000737:chemistry*; D033363:Neutron Diffraction / Q000379:methods*; D044367:Phase Transition; D013113:Spin Labels; D013696:Temperature
chemical_list: D013113:Spin Labels; D008187:Lutetium